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http://hdl.handle.net/10773/19362
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DC Field | Value | Language |
---|---|---|
dc.contributor.author | Peres, M. | pt |
dc.contributor.author | Magalhaes, S. | pt |
dc.contributor.author | Soares, M. R. | pt |
dc.contributor.author | Soares, M. J. | pt |
dc.contributor.author | Rino, L. | pt |
dc.contributor.author | Alves, E. | pt |
dc.contributor.author | Lorenz, K. | pt |
dc.contributor.author | Correia, M. R. | pt |
dc.contributor.author | Lourenco, A. C. | pt |
dc.contributor.author | Monteiro, T. | pt |
dc.date.accessioned | 2017-12-07T19:10:08Z | - |
dc.date.issued | 2013 | pt |
dc.identifier.issn | 1862-6351 | pt |
dc.identifier.uri | http://hdl.handle.net/10773/19362 | - |
dc.description.abstract | In this work ZnO thin films were deposited on different substrates, glass, silicon (100), and MgO (100) using rf-magnetron sputtering at low temperature in order to promote a large defect density, aiming to study a possible correlation with the observed violet/blue emission band. The peak position, width and low energy band shape asymmetry of the violet/blue band was found to be dependent on the deposition temperature and oxygen partial pressure. The structural analysis of deposited films reveals an epitaxial relationship for the a-oriented ZnO/MgO while for the c-oriented ZnO/Si no epitaxial relation was found with the substrate. The dependence of the violet/blue band on temperature displays always a shift of the peak position to lower energies, discarding the hypothesis of a free to bound transition. The sublinear dependence of the emission intensity with the excitation intensity suggests that the violet/blue bands on both samples could have a donor-acceptor pair nature. However, the unusually strong shift of the peak position to lower energies for the ZnO/MgO films and the emphasised asymmetric band shape for the ZnO/Si samples suggest that potential fluctuations in the electronic bands, due to disorder induced charged defects, could also be considered as an alternative recombination model for the violet/blue band. (C) 2013 WILEY-VCH Verlag GmbH \& Co. KGaA, Weinheim | pt |
dc.language.iso | eng | pt |
dc.publisher | WILEY-V C H VERLAG GMBH | pt |
dc.relation | info:eu-repo/grantAgreement/FCT/3599-PPCDT/100756/PT | pt |
dc.relation | info:eu-repo/grantAgreement/FCT/SFRH/SFRH%2FBD%2F45774%2F2008/PT | pt |
dc.relation | info:eu-repo/grantAgreement/FCT/SFRH/SFRH%2FBD%2F44635%2F2008/PT | pt |
dc.relation | info:eu-repo/grantAgreement/FCT/COMPETE/132936/PT | pt |
dc.rights | restrictedAccess | por |
dc.subject | PHOTOLUMINESCENCE | pt |
dc.subject | BLUE | pt |
dc.subject | SEMICONDUCTORS | pt |
dc.subject | GLASS | pt |
dc.subject | GAP | pt |
dc.title | Disorder induced violet/blue luminescence in rf-deposited ZnO films | pt |
dc.type | article | pt |
dc.peerreviewed | yes | pt |
ua.distribution | international | pt |
degois.publication.firstPage | 662 | pt |
degois.publication.issue | 4 | pt |
degois.publication.lastPage | 666 | pt |
degois.publication.title | PHYSICA STATUS SOLIDI C: CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 10, NO 4 | pt |
degois.publication.volume | 10 | pt |
dc.date.embargo | 10000-01-01 | - |
dc.relation.publisherversion | 10.1002/pssc.201200873 | pt |
dc.identifier.doi | 10.1002/pssc.201200873 | pt |
Appears in Collections: | CICECO - Artigos |
Files in This Item:
File | Description | Size | Format | |
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Disorder induced violetblue luminescence in rf-deposited ZnO films_10.1002pssc.201200873.pdf | 448.4 kB | Adobe PDF |
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